There are many buses between Mostar and Split - I've found 10 departures between Split and Mostar between 6am and 9pm. (Sorry, I couldn't find the schedules from Mostar to Split, but they run in intervals of almost every one to two hours). Just be careful in Mostar since buses use different locations for departures - besides Central bus station some buses also depart from the western part of the town. (Just cross the bridge opposite the Bus station and walk till the end of the street). Buses that go via Capljina, Metkovic and Ploce usually take at least 1,5 hour longer, although you can get some nice views along the way. Train is not an option between Mostar and Split.
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