Brasilia is a reputable bus company of Colombia. I try to avoid bus travel by night as much as possible in Colombia and Peru and never crossed the borders by land (as mentioned in your other posting). Be careful and keep a low profile. Be prepared for road blocks and checking for IDs by police/military several times (at least in Colombia; don't know about Venezuela).
The frontier area can be troublesome because of drug related activities and assumed guerilla presence (and their combination); Colombia accuses Venezuela of helping/giving shelter to those groups.
Good luck and happy travels
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